OK, for the time being I dialed it back to 3.6 GHz and auto-vcore, which seems to be stable.
I have no idea how I would go about screencapping my BIOS, so I just wrote down pretty much all the settings. I know some of them will be irrelevant, but better to be thorough than go through that tedium again

CPU Internal Cache: Enabled
Quick Power On Self Test: Enabled
APIC Mode: Enabled
MPS Version Control for OS: 1.4
CPU Multiplier: 9X
FSB - Memory Clock Mode: Unlinked
FSB (QDR), MHz: 1600
MEM (DDR), MHz: 1333
P1: Auto
P2: Auto
Memory Timing Setting: Expert
tCL: 7
tRCD: 7
tRP: 7
tRAS: 20
Command Per Clock: 1T
tRRD: Auto(4)
tRC: Auto(33)
tWR: Auto(12)
tWTR: Auto(16)
tFAW: Auto(21)
tREF: Auto(7.7uS)
tRFC: Auto(74)
PCIe x16_1 & x16_2, MHz: Auto(100)
PCIe x16_3, MHz: Auto(100)
SPP<->MCP Ref Clock, MHz: Auto(200)
HT Multiplier:
nForce SPP --> nForce MCP: 5x
nForce SPP <-- nForce MCP: 5x
HT Spread Spectrum: Auto
PCIe Spread Spectrum(SPP): Disabled
PCIe Spread Spectrum(MCP): Auto
SATA Spread Spectrum: Disabled
Limit CPUID MaxVal: Disabled
Intel SpeedStep: Disabled
CPU Thermal Control: Disabled
CE Enhanced Halt State: Disabled
Execute Disable Bit: Enabled
Virtualization Technology: Enabled
Voltages:
CPU Core: Auto(1.31V)
CPU FSB: Auto(1.3V)
Memory: 1.65V
nForce SPP: Auto(1.35V)
nForce MCP: Auto(1.5V)
GTLVREF Lanes 0-3: Auto(+00mv)
NVMEM memory test: Disable
OS Comp: Auto
System BIOS Cacheable: Disabled
HPET Function: Enabled
IEEE1394 Controller: Enabled
JMicron AHCI Controller: Enabled
HD Audio: Auto
IDE HDD Block MOde: Enabled
Onboard FDC Controller: Enabled
Onboard Serial Port 1: 3F8/IRQ4
ACPI function: Enabled
ACPI Suspend Type: S3(STR)
Soft-Off by PBTN: Instant-Off
WOL(PME#) From Soft-Off: Disabled
WOL(RI#) From Soft-Off: Disabled
PWRON After PWR-Fail: Off
Power-On by Alarm: Disabled
POWER ON Function: BUTTON ONLY
Init Display First: PCI Slot
Reset Configuration Data: Disabled
REsources Controlled By: Auto(ESCD)
PCI/VGA Palette Snoop: Disabled
PCI Latency Timer(CLK): 32
Maximum Payload Size: 4096